Terrestrial Methane Cycling During Paleogene Greenhouse Climates (NERC grant NE/J008591/1)
Supplementary material for published paper, Early Paleogene wildfires in peat-forming environments at Schoningen, Germany by BE Robson et al, http://doi.org/10.1016/j.palaeo.2015.07.016 NERC grant abstract: Human activity has led to an increase in pCO2 and methane levels from pre-industrial times to today. While the former increase is primarily due to fossil fuel burning, the increase in methane concentrations is more complex, reflecting not only direct human activity but also feedback mechanisms in the climate system related to temperature and hydrology-induced changes in methane emissions. To unravel these complex relationships, scientists are increasingly interrogating ancient climate systems. Similarly, one of the major challenges in palaeoclimate research is understanding the role of methane biogeochemistry in governing the climate of ice-free, high-pCO2 greenhouse worlds, such as during the early Paleogene (around 50Ma). The lack of proxies for methane concentrations is problematic, as methane emissions from wetlands are governed by precipitation and temperature, such that they could act as important positive or negative feedbacks on climate. In fact, the only estimates for past methane levels (pCH4) arise from our climate-biogeochemistry simulations wherein GCMs have driven the Sheffield dynamic vegetation model, from which methane fluxes have been derived. These suggest that Paleogene pCH4 could have been almost 6x modern pre-industrial levels, and such values would have had a radiative forcing effect nearly equivalent to a doubling of pCO2, an impact that could have been particularly dramatic during time intervals when CO2 levels were already much higher than today's. Thus, an improved understanding of Paleogene pCH4 is crucial to understanding both how biogeochemical processes operate on a warmer Earth and understanding the climate of this important interval in Earth history. We propose to improve, expand and interrogate those model results using improved soil biogeochemistry algorithms, conducting model sensitivity experiments and comparing our results to proxy records for methane cycling in ancient wetlands. The former will provide a better, process-orientated understanding of biogenic trace gas emissions, particularly the emissions of CH4, NOx and N2O. The sensitivity experiments will focus on varying pCO2 levels and manipulation of atmospheric parameters that dictate cloud formation; together, these experiments will constrain the uncertainty in our trace greenhouse gas estimates. To qualitatively test these models, we will quantify lipid biomarkers and determine their carbon isotopic compositions to estimate the size of past methanogenic and methanotrophic populations, and compare them to modern mires and Holocene peat. The final component of our project will be the determination of how these elevated methane (and other trace gas) concentrations served as a positive feedback on global warming. In combination our work will test the hypothesis that elevated pCO2, continental temperatures and precipitation during the Eocene greenhouse caused increased wetland GHG emissions and atmospheric concentrations with a significant feedback on climate, missing from most modelling studies to date. This work is crucial to our understanding of greenhouse climates but such an integrated approach is not being conducted anywhere else in the world; here, it is being led by international experts in organic geochemistry, climate, vegetation and atmospheric modelling, and palaeobotany and coal petrology. It will represent a major step forward in our understanding of ancient biogeochemical cycles as well as their potential response to future global warming.
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http://doi.org/10.1016/j.palaeo.2015.07.016
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http://www.bgs.ac.uk/services/ngdc/accessions/index.html#item75289
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http://data.bgs.ac.uk/id/dataHolding/13607142
eng
NERC grant, lead NE/J008591/1, associated grants NE/J008656/1 and NE/J00748X/1
geoscientificInformation
publication
2008-06-01
Lignite
Eocene
Charcoal
Inertinite
Coal
revision
2011
NERC_DDC
2012-09-01
2016-02-29
publication
2015-07
notApplicable
Lineage information may be available in the published paper, http://doi.org/10.1016/j.palaeo.2015.07.016
publication
2011
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See the referenced specification
publication
2010-12-08
false
See http://eur-lex.europa.eu/LexUriServ/LexUriServ.do?uri=OJ:L:2010:323:0011:0102:EN:PDF
The copyright of materials derived from the British Geological Survey's work is vested in the Natural Environment Research Council [NERC]. No part of this work may be reproduced or transmitted in any form or by any means, or stored in a retrieval system of any nature, without the prior permission of the copyright holder, via the BGS Intellectual Property Rights Manager. Use by customers of information provided by the BGS, is at the customer's own risk. In view of the disparate sources of information at BGS's disposal, including such material donated to BGS, that BGS accepts in good faith as being accurate, the Natural Environment Research Council (NERC) gives no warranty, expressed or implied, as to the quality or accuracy of the information supplied, or to the information's suitability for any use. NERC/BGS accepts no liability whatever in respect of loss, damage, injury or other occurence however caused.
School of Chemistry
University of Bristol
Bristol
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British Geological Survey
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2022-05-25